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I want him to make that mistake.
This is a good way to look at it. By check raising, you make that mistake more expensive with the exceptions noted above. Also note that check 3 betting makes their mistake of calling three bets cold an even bigger mistake. You're giving your the opportunity to either fold their equity or pay to realize that equity. Great no limit holdem players are especially good at knowing just how much to bet in order to either get a call or a fold. We don't have the option of mixing our betsizes in limit holdem, but we can make our opponent's mistakes more expensive by getting them to put in the most possible bets when we have big hands.
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The way he called on the flop and turn, I thought he was on a heart draw, not AJ for the gutshot.
I'm not really a fan of putting people on specific hands, unless ranges actually get so narrow that I think they have exactly one hand. For example, I was playing uncapped limit holdem online and made a set with QQ on the KQ2r board. No flush by the river and of course my opponent wants to keep raising. I reraised a few times but eventually called expecting to see KK the majority of the time. Yup he had KK.
Another time my opponent cold capped the A63 J turncard when I had 33. Ace on the river and I just call totally expecting to see AJ. Yup he had AJ.
In these spots, my opponent's ranges had become so narrow that I could put them on specific hands. Without the action to tell me that I was beat, my hands were monsters.
Usually, you can't be so sure as to what your opponent is holding. It would be nice if we all could think about ranges fluently at game speed, but realistically, many of us can't. If this is the case and you need to focus on a specific hand, I suggest thinking about where your opponent puts the "good hand/bad hand" threshold. For example, if I was on the button I would put your "good hand/bad hand" threshold somewhere around KTs for betting this flop. Yup, I put you on KTs and anything better, maybe throw in the occasional JTs for the open ended straight draw. I think you would check anything worse. Then when the action comes to me, I'm gonna estimate my equity vs your betting range. I'm gonna raise when I think I have enough equity to jam and I'm gonna call when I think I have enough equity to bluffcatch and draw. I'll fold if I don't think I have enough equity to do either.